Integer charge transfer at the tetrakis(dimethylamino)ethylene/Au interface

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Lindell, L. and Unge, M. and Osikowicz, W. and Stafstrom, S and Salaneck, W.R. and Crispin, X. and Jong, M.P. de (2008) Integer charge transfer at the tetrakis(dimethylamino)ethylene/Au interface. Applied physics letters, 92 . p. 163302. ISSN 0003-6951

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Abstract:In organic-based electronics, interfacial properties have a profound impact on device performance.
The lineup of energy levels is usually dependent on interface dipoles, which may arise from charge
transfer reactions. In many applications, metal-organic junctions are prepared under ambient
conditions, where direct overlap of the organic system from the metal bands is prevented due to
presence of oxides and/or hydrocarbons. We present direct experimental and theoretical evidence
showing that the interface energetic for such systems is governed by exchange of an integer amount
of electrons.
Item Type:Article
Copyright:© 2008 American Institute of Physics
Faculty:
Electrical Engineering, Mathematics and Computer Science (EEMCS)
Research Group:
Link to this item:http://purl.utwente.nl/publications/62522
Official URL:http://dx.doi.org/10.1063/1.2912818
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Metis ID: 252097