Methane activation on a La0.6Sr0.4Co0.8Fe0.2O3 perovskite: Catalytic and electrocatalytic results

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Tsiakaras, P. and Athanasiou, C. and Marnellos, G. and Stoukides, M. and Elshof, J.E. ten and Bouwmeester, H.J.M. (1998) Methane activation on a La0.6Sr0.4Co0.8Fe0.2O3 perovskite: Catalytic and electrocatalytic results. Applied Catalysis A: General, 169 (2). pp. 249-261. ISSN 0926-860X

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Abstract:The catalytic and electrocatalytic behavior of the La0.6Sr0.4Co0.8Fe0.2O3 (LSCF) perovskite deposited on yttria-stabilized zirconia (YSZ) was studied during the reaction of methane oxidation. Experiments were carried out in a well-mixed (CSTR) reactor at atmospheric pressure, in the 600–900°C range. When, instead of co-feeding with methane in the gas phase, oxygen was electrochemically supplied as O2−, considerable changes in the methane conversion and product selectivity were observed. Catalytic and electrocatalytic results were compared to those obtained when the LSCF served as a dense mixed-conducting membrane supplying oxygen to the methane feed stream because of the oxygen partial-pressure gradient across the membrane.
Item Type:Article
Copyright:Elsevier Science
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Science and Technology (TNW)
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Link to this item:http://purl.utwente.nl/publications/61709
Official URL:http://dx.doi.org/10.1016/S0926-860X(98)00013-1
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